Photoelectrochemical Water Splitting: Materials, Processes by Hans-Joachim Lewerenz, Laurie Peter, Ferdi Schüth, Tim Zhao, PDF

By Hans-Joachim Lewerenz, Laurie Peter, Ferdi Schüth, Tim Zhao, Heinz Frei, Bruce Parkinson, John Turner, Nathan Lewis, Kevin Sivula, Kazunari Domen, Allen J Bard, Sebastian Fiechter, Ramon Collazo, Thomas Hannappel, Anders Hellman, Krishnan Rajeshwar, Marc

A quantity that may offer a accomplished assessment of present task within the box of photoelectrochemistry that's contributing more and more to the improvement of novel ideas, fabrics and techniques that may be used for the construction of sunlight fuels. themes coated will contain: points of photoelectrochemical water splitting;  combinatorial method of fabrics discovery for water splitting; mesoporous transition steel oxides for water splitting; tandem photoelectrochemical cells for water splitting; nano-architectures for sun  water splitting units; microheterogeneous photocatalysts for water splitting; effective III-V architectures for H2O splitting; the III-V nitride kin; coupled electron proton move; computational insights into O2-evolving advanced of PSII; hydrogen evolution; floor research of molecular adsorbates on oxides; interfacial kinetics; floor research of catalysts and absorbers; biomimetic platforms and catalysts; multi-electron move; molecular catalysts for sun fuels; 3rd iteration units; plasmonics; power move; and destiny improvement horizons.

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The dependence of Csc on the potential drop across the space charge region (Dfsc) is given by the Mott–Schottky equation (here for an n-type electrode) ! 1 2 kB T ¼ Dfsc À ð2:2Þ 2 Csc Nd ee0 q For low or moderately doped semiconductors under depletion conditions, CHcCsc, so that it is often assumed that changes in electrode potential appear mainly across the space charge region. In this case, Dfsc can be replaced by U – Ufb, where U is the applied potential. However, for many of the materials that are studied in the context of water splitting, this approximation may not be valid for several reasons.

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